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Synthesis of Ionic Liquid Based Electrolytes, Assembly of Li-ion Batteries, and Measurements of Performance at High Temperature
Published on: December 20, 2016
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Enabling High-Temperature and High-Voltage Lithium-Ion Battery Performance through a Novel Cathode Surface-Targeted
Noah M Johnson1, Zhenzhen Yang1, Ira Bloom1
1Chemical Sciences and Engineering Division, Argonne National Laboratory, 9700 S. Cass Ave., Lemont, Illinois 60439, United States.
ACS Applied Materials & Interfaces
|December 3, 2021
Summary
Researchers developed a novel additive to stabilize lithium-ion battery positive electrodes against high temperatures and voltages. This breakthrough enhances battery performance and longevity in demanding applications.
Area of Science:
- Materials Science
- Electrochemistry
- Energy Storage
Background:
- Lithium-ion batteries (LIBs) face increasing demands for stability across diverse operating conditions.
- Stabilizing negative electrodes in LIBs is well-studied, but positive electrode stabilization remains a significant challenge.
- Broader LIB applications necessitate improved performance under extreme temperatures and voltages.
Purpose of the Study:
- To develop a novel additive for enhancing the stability of positive electrodes in lithium-ion batteries.
- To address the limitations of current electrolyte development in stabilizing positive electrodes.
- To improve the operational safety and longevity of LIBs under harsh conditions.
Main Methods:
- Introduction of a novel chemical additive into the battery electrolyte.
- Electrochemical testing of LIBs with the additive under elevated temperatures and voltages.
- Analysis of additive functionality within complex electrolyte systems.
Main Results:
- The novel additive effectively protected positive electrodes against degradation at elevated temperatures and voltages.
- The additive demonstrated efficacy even when used in small quantities.
- The additive maintained functionality within complex electrolyte formulations.
Conclusions:
- A new additive offers a targeted solution for stabilizing lithium-ion battery positive electrodes.
- This approach can significantly improve LIB performance and reliability in demanding applications.
- The additive represents a promising strategy for advancing energy storage technology.

