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Updated: Oct 8, 2025

High-Temperature and High-Pressure In situ Magic Angle Spinning Nuclear Magnetic Resonance Spectroscopy
Published on: October 9, 2020
Spatially resolved optical spectroscopy in extreme environment of low temperature, high magnetic fields and high
I Breslavetz1, A Delhomme1, T Pelini1
1LNCMI, UPR 3228, CNRS, EMFL, Université Grenoble Alpes, 38000 Grenoble, France.
Abstract:
We present an experimental setup developed to perform optical spectroscopy experiments (Raman scattering and photoluminescence measurements) with a micrometer spatial resolution in an extreme environment of low temperature, high magnetic field, and high pressure. This unique experimental setup, to the best of our knowledge, allows us to deeply explore the phase diagram of condensed matter systems by independently tuning these three thermodynamic parameters while monitoring the low-energy excitations (electronic, phononic, or magnetic excitations) to spatially map the Raman scattering response or to investigate objects with low dimensions. We apply this technique to bulk FePS3, a layered antiferromagnet with a Néel temperature of T ≈ 120 K.
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