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Suppression of Photoinduced Phase Segregation in Mixed-Halide Perovskite Nanocrystals for Stable Light-Emitting
Feixiang Xu1,2,3, Dejian Chen2,3,4, Decai Huang2,3,4
1Department of Optoelectronic and Communication Engineering, Xiamen University of Technology, Xiamen, Fujian 361024, China.
Abstract:
Halide segregation is a critical bottleneck that hampers the application of mixed-halide perovskite nanocrystals (NCs) in both electroluminescent and down-conversion red-light-emitting diodes. Herein, we report a strategy that combines precursor and surface engineering to obtain pure-red-emitting (peaked at 624 nm) NCs with a photoluminescence quantum yield of up to 92% and strongly suppresses the halide segregation of mixed-halide NCs under light irradiation. Red-light-emitting diodes (LED) using these mixed-halide NCs as phosphors exhibit color-stable emission with a negligible peak shift and spectral broadening during operation over 240 min. By contrast, a dramatic peak shift and spectral broadening were observed after 10 min of operation in LEDs based on mixed-halide NCs synthesized by a traditional method. Our strategy is critical to achieving photo- and band-gap-stable mixed-halide perovskite NCs for a variety of optoelectronic applications such as micro-LEDs.
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