Longitudinal assessment of personal air pollution clouds in ten home and office environments

Elevated exposure to indoor air pollution is associated with negative human health and well-being outcomes. Inhalation exposure studies commonly rely on stationary monitors in combination with human time-activity patterns; however, this method is susceptible to exposure misclassification. We tracked ten participants during five consecutive workdays with stationary air pollutant monitors at their homes and offices, and wearable personal monitors. Real-time measures of size-resolved particulate matter (within range 0.3-10 μm) and CO₂ , and integrated samples of PM₁₀ , VOCs, and aldehydes were collected. The PM₁₀  cloud magnitude (excess of PM₁₀ beyond stationary room concentration) was detected for all participants in homes and offices. The PM₁₀  cloud magnitude ranged within 5-37 μg/m³ and was the most discernible in the coarse particle size fraction. Particles associated with "Urban mix," "Traffic," and "Human activities" sources contributed the most to PM₁₀ exposures. The personal CO₂  clouds were detected for participants with the SEMs in their living rooms and private or low-occupancy offices. The stationary monitors placed in bedrooms were better predictors of personal PM₁₀ and CO₂ exposures. An overall of 33 VOCs and aldehydes were detected in both microenvironments, with the majority exhibiting high correlation between personal and stationary stations.