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Updated: Sep 25, 2025

Flame Experiments at the Advanced Light Source: New Insights into Soot Formation Processes
Published on: May 26, 2014
In situ temperature measurements in sooting methane/air flames using synchrotron x-ray fluorescence of seeded krypton
Matthew J Montgomery1, Hyunguk Kwon2, Alan L Kastengren3
1Department of Chemical and Environmental Engineering, Yale University, New Haven, CT, USA.
Abstract:
Synchrotron x-ray fluorescence has been used to measure temperatures in optically dense gases where traditional methods would fail. These data provide a benchmark for stringent tests of computational fluid dynamics models for complex systems where physical and chemical processes are intimately linked. The experiments measured krypton number densities in a sooting, atmospheric pressure, nonpremixed coflow flame that is widely used in combustion research. The experiments not only form targets for the models, but the simulations also identify potential sources of uncertainties in the measurements, allowing for future improvements.
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