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A thermo-reversible silicone elastomer with remotely controlled self-healing.

E Ogliani1, L Yu1, I Javakhishvili1

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Summary

This study introduces a novel, recyclable silicone elastomer that is self-healing and stimuli-responsive. This advanced material offers enhanced durability and reliability for demanding applications.

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Area of Science:

  • Materials Science
  • Polymer Chemistry

Background:

  • Soft thermoplastic elastomers are highly sought after for their durability and reliability.
  • Silicone elastomers, while soft and durable, lack thermoplasticity and can fail under extreme conditions.

Purpose of the Study:

  • To develop a thermo-reversible, self-healing, and recyclable silicone-based elastomer.
  • To overcome the limitations of conventional silicone elastomers.

Main Methods:

  • Incorporation of supramolecular 2-ureido-4[1H]-pyrimidone (UPy) self-assembling motifs via free radical polymerization.
  • Stimuli-responsivity achieved through UPy motifs and incorporation of Fe3O4 particles for magnetic field-triggered self-healing.

Main Results:

  • The novel elastomer exhibits self-healing properties triggered by direct or indirect heating (magnetic field).
  • The material demonstrates excellent recyclability due to temperature responsiveness and high thermal stability, withstanding multiple reprocessing cycles.
  • The developed elastomer maintains its properties after repeated processing.

Conclusions:

  • The novel silicone-based elastomer offers a unique combination of self-healing, recyclability, and stimuli-responsiveness.
  • This material presents a promising solution for applications requiring soft, reliable, and durable elastomers.
  • The developed material is suitable for various applications demanding high performance under extreme conditions.