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Methods of Ex Situ and In Situ Investigations of Structural Transformations: The Case of Crystallization of Metallic Glasses
Published on: June 7, 2018
Mean-field description for the architecture of low-energy excitations in glasses
Wencheng Ji1, Tom W J de Geus1, Elisabeth Agoritsas1
1Institute of Physics, École Polytechnique Fédérale de Lausanne (EPFL), CH-1015 Lausanne, Switzerland.
Abstract:
In amorphous materials, groups of particles can rearrange locally into a new stable configuration. Such elementary excitations are key as they determine the response to external stresses, as well as to thermal and quantum fluctuations. Yet, understanding what controls their geometry remains a challenge. Here we build a scaling description of the geometry and energy of low-energy excitations in terms of the distance to an instability, as predicted, for instance, at the dynamical transition in mean-field approaches of supercooled liquids. We successfully test our predictions in ultrastable computer glasses, with a gapped spectrum and an ungapped (regular) spectrum. Overall, our approach explains why excitations become less extended, with a higher energy and displacement scale upon cooling.
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