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Generalised non-negative matrix factorisation for air pollution source apportionment.

Nirav L Lekinwala1, Mani Bhushan2

  • 1Department of Chemical Engineering, Indian Institute of Technology Bombay, Mumbai 400076, Maharashtra, India.

The Science of the Total Environment
|June 1, 2022
PubMed
Summary

This study introduces Generalised Non-Negative Matrix Factorisation (GNMF) for air pollution source apportionment. GNMF accurately accounts for correlated errors in data, improving upon existing methods like Positive Matrix Factorisation (PMF).

Keywords:
Correlated errorsMultiplicative updateProjected gradient approachReceptor modeling

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Area of Science:

  • Environmental Science
  • Analytical Chemistry
  • Data Science

Background:

  • Source Apportionment (SA) is crucial for air pollution control policy.
  • Positive Matrix Factorisation (PMF) is a common SA technique but assumes uncorrelated errors.
  • Existing Non-Negative Matrix Factorisation (NMF) methods have restrictive assumptions on error structures.

Purpose of the Study:

  • To develop a novel SA method that incorporates general error covariance structures.
  • To address the limitation of uncorrelated error assumptions in existing SA techniques.
  • To introduce Generalised Non-Negative Matrix Factorisation (GNMF) for improved SA.

Main Methods:

  • Developed Generalised Non-Negative Matrix Factorisation (GNMF) by integrating the full error covariance matrix into the objective function.
  • Derived iterative update rules for factor matrices (G and F).
  • Extended existing NMF techniques (multiplicative and projected gradient) to ensure non-negativity in GNMF.

Main Results:

  • The proposed GNMF method can handle any error covariance matrix without restrictive assumptions.
  • GNMF subsumes various existing NMF methods as special cases.
  • Demonstrated the effectiveness of GNMF on a field measurement dataset for SA.

Conclusions:

  • GNMF offers a more robust and flexible approach to Source Apportionment compared to traditional methods.
  • The ability to incorporate general error structures enhances the accuracy of identifying pollution sources.
  • GNMF provides a valuable tool for environmental policy development by improving air pollution source identification.