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Oxygen functionalized hexagonal boron nitride (hBN) exhibits significant magneto-optical Kerr effects. This 2D material shows potential for designing advanced magneto-optical devices, even at high temperatures.

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Area of Science:

  • Condensed Matter Physics
  • Materials Science
  • Nanotechnology

Background:

  • Atomically thin functional materials are crucial for exploring 2D magneto-optics.
  • Magneto-optical experimental data show significant Kerr signals in insulator thin films.

Purpose of the Study:

  • Investigate the magneto-optical Kerr effect in oxygen functionalized and doped hexagonal boron nitride (hBN).
  • Calculate Kerr angle and Kerr ellipticity for functionalized hBN.
  • Explore the impact of oxygen doping on hBN's properties.

Main Methods:

  • First-principles calculations were employed to study the magneto-optical Kerr effect.
  • Kerr angle and Kerr ellipticity were computed for functionalized hBN.

Main Results:

  • Functionalized hBN demonstrates significant magneto-optical Kerr signals.
  • Increasing oxygen doping introduces surface plasmon resonance in hBN.
  • Functionalized hBN maintains structural integrity (bridge-bonded oxygen) at high temperatures.

Conclusions:

  • Functionalized hBN exhibits giant opto/magnetic responses, suitable for insulating 2D materials.
  • These findings offer a platform for designing novel magneto-optical devices.