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Updated: Sep 5, 2025

Direct Imaging of Laser-driven Ultrafast Molecular Rotation
Published on: February 4, 2017
The time-resolved atomic, molecular and optical science instrument at the Linac Coherent Light Source
Peter Walter1, Timur Osipov1, Ming Fu Lin1
1SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, CA 94025, USA.
The new time-resolved atomic, molecular, and optical science instrument (TMO) leverages two SLAC accelerators for advanced soft X-ray free-electron laser experiments. This flexible setup enables novel studies in ultrafast electronic and molecular phenomena.
Area of Science:
- Atomic, Molecular, and Optical (AMO) Science
- Ultrafast Science
- Soft X-ray Physics
Background:
- The need for advanced experimental capabilities in AMO science.
- Limitations of previous instruments at SLAC.
- The potential of soft X-ray free-electron lasers.
Purpose of the Study:
- Introduce the newly constructed Time-Resolved Atomic, Molecular, and Optical science instrument (TMO).
- Highlight TMO's unique capabilities and flexibility.
- Expand experimental possibilities at the SLAC National Accelerator Laboratory.
Main Methods:
- Utilizing two linear accelerators: a copper accelerator (120 Hz) for high per-pulse energy and a superconducting accelerator (1 MHz) for high average intensity.
- Employing a soft X-ray free-electron laser with a variable-gap undulator.
- Implementing two in-line X-ray beam focus spots and a dynamic reaction microscope with a sub-micrometer focus.
Main Results:
- TMO supports a wide range of experimental techniques previously unavailable at LCLS.
- The instrument is optimized for studying ultrafast electronic and molecular phenomena.
- Sub-femtosecond soft X-ray pulse generation is fully leveraged.
Conclusions:
- The TMO instrument significantly enhances research capabilities in AMO science and ultrafast phenomena.
- Its flexible design and advanced light source enable novel investigations.
- TMO opens new avenues for studying dynamic reactions and electronic processes at the femtosecond timescale.
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