Strong mode coupling-enabled hybrid photon-plasmon laser with a microfiber-coupled nanorod

Laser based on single plasmonic nanoparticle can provide optical frequency radiation far beyond the diffraction limit and is one of the ultimate goals of nanolasers, yet it remains a challenge to be realized because of the inherently high Ohmic loss. Here, we report the direct observation of lasing in microfiber-coupled single plasmonic nanoparticles enabled by strong mode coupling. We show that, by strongly coupling a gold nanorod (GNR) with the whispering gallery cavity of a dye-doped polymer microfiber (with diameter down to 2.0 μm), the substantially enhanced optical coherence of the hybrid photon-plasmon mode and effective gain accumulated from the active microfiber cavity enable single-mode laser emission from the GNR at room temperature with a threshold as low as 2.71 MW/cm² and a linewidth narrower than 2 nm.