Photodetection and Infrared Imaging Based on Cd₃As₂ Epitaxial Vertical Heterostructures

Due to the nontrivial electronic structure, Cd₃As₂ is predicted to possess various transport properties and outstanding photoresponses. Photodetectors based on topological materials are mostly made up of nanoplates, yet monolithic in situ heteroepitaxial Cd₃As₂ photodetectors are rarely reported to date owing to the crystal mismatch between Cd₃As₂ and semiconductors. Here, we demonstrate Cd₃As₂/ZnCd_1-Te/GaSb vertical heteroepitaxial photodetectors via molecule beam epitaxy. By constructing dual-Schottky junctions, these photodetectors show high responsivity and external quantum efficiency in a broadband spectrum. Based on the strong and fast photoresponse, we achieved visible light to near-infrared imaging using a one-pixel imaging system with a galvo. Our results illustrate that the integration of three-dimensional Dirac semimetal Cd₃As₂ with semiconductors has potential applications in broadband photodetection and infrared cameras.