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Phase-field numerical study on the dynamic process of thermocapillary patterning.

Qingzhen Yang1,2,3,4, Yankui Liu5, Xinmiao Jia1,2

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Nonuniform temperatures drive thermocapillary flow (Marangoni effect), enabling precise micro- and nanostructure fabrication via thermocapillary patterning. This study models the dynamic process and parameter influences for advanced material structuring.

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Area of Science:

  • Fluid Dynamics
  • Materials Science
  • Surface Physics

Background:

  • Surface tension is temperature-dependent, leading to thermocapillary flow (Marangoni effect) when temperature gradients exist.
  • Thermocapillary patterning utilizes this effect to deform thin liquid films, creating micro- and nanostructures that often replicate template topography.

Purpose of the Study:

  • To develop and employ a numerical model for studying the dynamic process of thermocapillary patterning.
  • To investigate the influence of key parameters on the thermocapillary patterning phenomenon.

Main Methods:

  • Development of a two-phase flow numerical model utilizing the phase field method.
  • The phase field approach allows seamless integration of thermal fields, multiphase flow, and free surface deformation without remeshing.

Main Results:

  • The numerical model successfully simulated the dynamic process of thermocapillary patterning.
  • Investigated the impact of temperature, geometric parameters, and contact angle on structure formation.

Conclusions:

  • The phase field-based numerical model is effective for studying thermocapillary patterning dynamics.
  • Understanding parameter effects is crucial for optimizing the fabrication of micro- and nanostructures using this technique.