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LiNi0.5Mn1.5O4 Cathode Microstructure for All-Solid-State Batteries.

Hyeon Jeong Lee1,2,3, Xiaoxiao Liu1,4, Yvonne Chart1,2

  • 1Department of Materials, University of Oxford, Oxford OX1 3PH, U.K.

Nano Letters
|September 7, 2022
PubMed
Summary
This summary is machine-generated.

Researchers developed hollow, Al2O3-coated LiNi0.5Mn1.5O4 particles for solid-state batteries. This novel cathode microstructure enhances stability and energy density, improving battery performance and longevity.

Keywords:
areal capacitiescathode microstructurehigh-voltage cathodesinterfacessolid-state batteries

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Energy Storage

Background:

  • Solid-state batteries (SSBs) offer higher energy density and safety than Li-ion batteries.
  • Practical SSBs face challenges like capacity decay due to poor electrode contact.
  • LiNi0.5Mn1.5O4 (LNMO) is a promising cathode material for high-voltage SSBs.

Purpose of the Study:

  • Investigate the impact of cathode microstructure on SSB performance.
  • Design and synthesize Al2O3-coated LNMO with a hollow structure.
  • Improve cathode utilization and cycling stability in SSBs.

Main Methods:

  • Synthesized Al2O3-coated hollow LNMO particles.
  • Fabricated SSB cells using Li6PS5Cl solid electrolyte.
  • Performed electrochemical cycling tests to evaluate capacity retention and stability.

Main Results:

  • Demonstrated improved cycling stability with the hollow LNMO cathode.
  • Achieved over 70% capacity retention after 100 cycles.
  • Showcased high active material loading (27 mg cm-2) at 0.8 mA cm-2.

Conclusions:

  • Cathode microstructure is critical for SSB performance.
  • Hollow, coated LNMO particles enhance electrolyte stability and Li+ diffusion.
  • This approach offers a pathway to practical, high-performance solid-state batteries.