Spatio-temporal analysis of PM_2.5 and policies in Northwestern South America

This paper analyzes the spatio-temporal variations, and exceedances of the PM_2.5 concentrations in Northwestern South America at different scales to assess the implemented policies and identify the involved phenomena. Through reanalysis and ground-based data, we found that high PM_2.5 levels in most cities of the region are caused by wildfires and local emissions, including the capital cities of Venezuela, Ecuador, Colombia, and Panamá. In-situ measurements suggest that the majority of the cities comply with the local but not with the WHO guidelines, indicating that local annual limits should be more restrictive. Two peaks in the daily variations of PM_2.5 (related to vehicle emissions) and also a steeper decrease around noon (associated with an increase in wind speed and in the boundary layer height) were identified. The trend-analysis shows that Bogotá and Medellín have a decreasing PM_2.5 annual-trend (between -0.8μgm^-3 and -1.7μgm^-3) that corresponds to effective policies. In contrast, Cali has a positive annual-trend (0.8μgm^-3) most likely because of Short-Range Transport produced by a northerly-flow from a highly polluted neighboring city, which also affects Cali's PM_2.5 diurnal cycle, or by local-dynamics. The exceedances show that the policies are working on an annual but not at a daily time-scale. These results serve as a first input for additional studies, with the aim of gaining a better understanding of the contaminant before adapting current policies or implementing new policies and measures that need to include a joint international, regional, and inter-city efforts regarding pollution transport.