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Printed Stretchable Graphene Conductors for Wearable Technology.

Laura S van Hazendonk1, Artur M Pinto1,2, Kirill Arapov1

  • 1Laboratory of Physical Chemistry and Center for Multiscale Electron Microscopy, Department of Chemical Engineering and Chemistry, Eindhoven University of Technology, P.O. Box 513, 5600MB Eindhoven, The Netherlands.

Chemistry of Materials : a Publication of the American Chemical Society
|September 19, 2022
PubMed
Summary
This summary is machine-generated.

Researchers developed a new graphene-based ink for printable stretchable conductors. This innovation enables durable, highly conductive materials for wearable electronics, even after significant stretching and repeated use.

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Area of Science:

  • Materials Science
  • Nanotechnology
  • Polymer Science

Background:

  • Developing skin-compatible printed stretchable conductors with both low gauge factor and high durability remains a significant challenge.
  • Existing materials often compromise conductivity, durability, or skin compatibility under strain.

Purpose of the Study:

  • To create a graphene nanoplatelet-based colloidal ink using a skin-compatible thermoplastic polyurethane (TPU) binder.
  • To achieve stretchable conductors with high conductivity and durability for wearable applications.

Main Methods:

  • Formulation of a graphene nanoplatelet-based colloidal ink with a tunable thermoplastic polyurethane (TPU) binder.
  • Printing conductors onto TPU substrates.
  • Post-printing treatments including thermal drying and photonic annealing.

Main Results:

  • Achieved stretchable conductors with conductivity maintained up to 100% strain.
  • Demonstrated high fatigue resistance under cyclic strains of 20-50%.
  • Sheet resistances as low as 34 Ω □-1 mil-1 after thermal drying, reduced to <10 Ω □-1 mil-1 via photonic annealing.
  • Preserved and tunable stretchability and fatigue resistance after photonic annealing.

Conclusions:

  • The developed graphene-TPU ink enables the fabrication of highly conductive, durable, and stretchable conductors via printing.
  • Scalable ink production, adjustable rheology, and tunable properties support high-volume manufacturing of stretchable wearables.
  • This advancement addresses key challenges in creating advanced electronic textiles and wearable devices.