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Dual-Mode-Driven Micromotor Based on Foam-like Carbon Nitride and Fe3O4 with Improved Manipulation and Photocatalytic
Kai Feng1, Jiang Gong1, Jinping Qu1,2
1Key Laboratory of Material Chemistry for Energy Conversion and Storage, Ministry of Education, Hubei Key Laboratory of Material Chemistry and Service Failure, Hubei Engineering Research Center for Biomaterials and Medical Protective Materials, Semiconductor Chemistry Center, School of Chemistry and Chemical Engineering, Huazhong University of Science and Technology, Wuhan 430074, China.
Abstract:
Micro/nanomotors have emerged as a vibrant research topic in biomedical and environmental fields due to their attractive self-propulsion as well as small-scale functionalities. However, single actuated micro/nanomotors are not adaptive in facing intricate natural and industrial environments. Herein, we propose a new dual-mode-driven micromotor based on foam-like carbon nitride (f-C3N4) with precipitated Fe3O4 nanoparticles, namely, Fe3O4/f-C3N4, powered by chemical/magnetic stimuli for rapid reduction of organic pollutants. The Fe3O4/f-C3N4 motor composed of a three-dimensional (3D) porous "foam-like" structure and precipitated Fe3O4 nanoparticles (ca. 50 nm) not only exhibits efficient photocatalytic performance under visible light but also shows versatile and programmable motion behavior under the control of external magnetic fields. The aggregation of the micromotor under an external rotating magnetic field further enhances the catalytic activity by the increased local catalyst concentration. Furthermore, the magnetic property endows the micromotor with easy recyclability. This study provides a novel dual-mode-driven micromotor for antibiotics removal with magnetic field and light-enhanced performance in industrial wastewater treatment at a low cost.
