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Updated: Aug 25, 2025

Direct Imaging of Laser-driven Ultrafast Molecular Rotation
Published on: February 4, 2017
All-optical sampling of ultrashort laser pulses based on perturbed transient grating
Abstract:
We propose and demonstrate an all-optical pulse sampling technique based on the transient grating (TG) procedure with perturbation, which provides a simple and robust manner to characterize an ultrashort laser pulse without employing a retrieval algorithm. In our approach, a two-orders weaker perturbation pulse perturbs the diffracted pulse from the TG, which is generated by another strong fundamental pulse. The modulation of the diffracted pulse energy directly represents the temporal profile of the perturbation pulse. We have successfully characterized few-cycle and multi-cycle pulses, which is consistent with the results verified by the widely employed frequency-resolved optical gating (FROG) method. Our method provides a potential way to characterize ultrashort laser waveform from the deep-UV to far-infrared region.

