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Updated: Aug 21, 2025

Elemental-sensitive Detection of the Chemistry in Batteries through Soft X-ray Absorption Spectroscopy and Resonant Inelastic X-ray Scattering
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Mapping and Modeling Physicochemical Fields in Solid-State Batteries.

Zhe-Tao Sun1, Jingying Zhou1, Yifan Wu1

  • 1University of Michigan-Shanghai Jiao Tong University Joint Institute, Shanghai Jiao Tong University, 800 Dongchuan Road, Shanghai 200240, China.

The Journal of Physical Chemistry Letters
|November 16, 2022
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Summary
This summary is machine-generated.

Solid-state batteries offer enhanced safety and energy density. Understanding multiphysics coupling through advanced characterization and modeling is key to unlocking their full potential.

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Chemical Engineering

Background:

  • Solid-state batteries promise higher safety and energy density than conventional lithium-ion batteries.
  • Replacing liquid electrolytes with solid-state electrolytes introduces complex physicochemical field couplings.

Purpose of the Study:

  • To provide an overview of multiphysics coupling in solid-state batteries.
  • To highlight the need for advanced experimental and theoretical methods for tracking coupled fields during battery cycling.

Main Methods:

  • Survey of existing experimental characterization techniques for solid-state batteries.
  • Review of theoretical modeling approaches for multiphysics coupling.

Main Results:

  • Current understanding of electrochemical, stress, crack, and thermal field evolution in solid-state batteries is discussed.
  • Existing characterization techniques and their limitations are identified.

Conclusions:

  • Development of experimental tools for concurrent multiphysics mapping is crucial.
  • Incorporating material plasticity into theoretical models is essential for advancing solid-state battery technology.