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Published on: March 24, 2019
High-Angular Momentum Excitations in Collinear Antiferromagnet FePS3.
Jan Wyzula1,2, Ivan Mohelský1, Diana Václavková1
1Laboratoire National des Champs Magnétiques Intenses, CNRS UPR3228, EMFL, Univ. Grenoble Alpes, Univ. Toulouse, Univ. Toulouse 3, INSA-T, Grenoble and Toulouse, F-38042, France.
Researchers studied the magnetic properties of FePS3, discovering a unique multipolar magnon. This excitation, a 4-magnon bound state, could lead to exotic magnetic states in materials with high magnetic anisotropy.
Area of Science:
- Condensed matter physics
- Magnetism
- Materials science
Background:
- FePS3 is a quasi-two-dimensional van der Waals antiferromagnet.
- Antiferromagnetic resonance modes are typical in easy-axis antiferromagnets.
Purpose of the Study:
- Investigate magneto-optical properties of FePS3.
- Characterize unusual magnetic excitations in FePS3.
- Explore potential exotic magnetic states.
Main Methods:
- Magneto-optical studies.
- Analysis of magnetic excitations and Zeeman splitting.
Main Results:
- Observed an excitation resembling antiferromagnetic resonance.
- This excitation exhibited a four-times larger Zeeman splitting than expected.
- Identified the excitation as a single-ion |S|=4 multipolar magnon (4-magnon bound state).
- The multipolar magnon corresponds to a full magnetic moment reversal of Fe2+ ions.
Conclusions:
- Multipolar magnons are a novel type of magnetic excitation.
- Condensation of multipolar magnons may create exotic states in large-spin, anisotropic materials.
- FePS3 serves as a model system for studying multipolar magnons.
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