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Interface Engineering Enables High-Performance Sb Anode for Sodium Storage.

Chang Liu1, Xin Fu1, Shuzhen Liao1

  • 1School of Chemistry and Chemical Engineering, Hunan Institute of Engineering, Xiangtan 411104, China.

Nanomaterials (Basel, Switzerland)
|January 21, 2023
PubMed
Summary
This summary is machine-generated.

Interface engineering enhances sodium-ion batteries (SIBs) by creating MOF-C-Sb anodes. This design boosts energy density and stability, overcoming limitations of traditional antimony-based materials for better energy storage.

Keywords:
Sbheterointerface engineeringsodium-ion batteries

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Nanotechnology

Background:

  • Heterointerface engineering is key to improving alkali-ion battery energy density.
  • Designing heterogeneous composites with abundant interfaces for sodium-ion batteries (SIBs) remains challenging.

Purpose of the Study:

  • To explore interface engineering for enhancing SIB anode performance.
  • To rationally design and construct Sb-based anode materials for high-performance electrochemical energy storage.

Main Methods:

  • Density functional theory (DFT) calculations guided material design.
  • Fabrication of a porous heterointerface MOF-C-Sb composite using MOF-C as support.
  • Electrochemical performance testing for sodium storage.

Main Results:

  • Interface engineering reduced the bandgap and Na ion migration barrier in Sb and Na3Sb.
  • The MOF-C-Sb anode demonstrated high reversible capacity (540.5 mAh g-1 at 0.1 A g-1).
  • The material exhibited excellent rate capability (515.9 mAh g-1 at 1.6 A g-1) and resolved Sb volume expansion issues.

Conclusions:

  • The heterointerface-engineered structure offers significant advantages for SIBs.
  • MOF-C-Sb composite shows superior electrochemical performance for sodium storage.
  • This work provides valuable insights for designing advanced Sb-based anodes for energy storage.