Segmented cylindrical vector beams for massively-encoded optical data storage

The possibility to achieve unprecedented multiplexing of light-matter interaction in nanoscale is of virtue importance from both fundamental science and practical application points of view. Cylindrical vector beams (CVBs) manifested as polarization vortices represent a robust and emerging degree of freedom for information multiplexing with increased capacities. Here, we propose and demonstrate massively-encoded optical data storage (ODS) by harnessing spatially variant electric fields mediated by segmented CVBs. By tight focusing polychromatic segmented CVBs to plasmonic nanoparticle aggregates, record-high multiplexing channels of ODS through different combinations of polarization states and wavelengths have been experimentally demonstrated with a low error rate. Our result not only casts new perceptions for tailoring light-matter interactions utilizing structured light but also enables a new prospective for ultra-high capacity optical memory with minimalist system complexity by combining CVB's compatibility with fiber optics.