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Solvent-molecule interaction induced gating of charge transport through single-molecule junctions

Zheng Tang1, Songjun Hou2, Qingqing Wu2

  • 1State Key Laboratory of Physical Chemistry of Solid Surfaces, Collaborative Innovation Center of Chemistry for Energy Materials (iChEM), College of Chemistry and Chemical Engineering, Xiamen University, Xiamen 361005, China.

Science Bulletin
|February 7, 2023
PubMed
Summary

Solvent polarity significantly tunes single-molecule junction conductance by altering molecular orbital energies. Gating effects depend on anchor group coupling strength, with weaker coupling showing greater sensitivity to solvent interactions.

Keywords:
Break junctionsMolecular electronicsSingle-molecule conductanceSolvent-induced gating

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