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2D Materials Boost Advanced Zn Anodes: Principles, Advances, and Challenges.

Songhe Zheng¹, Wanyu Zhao¹, Jianping Chen¹

¹School of Materials Science and Engineering, Tongji University, Shanghai, 201804, People's Republic of China.

Nano-Micro Letters

|February 8, 2023

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Two-dimensional materials offer solutions for stable aqueous zinc-ion battery anodes, addressing dendrites and corrosion. This review guides the rational design of these advanced materials for practical energy storage applications.

Area of Science:

Materials Science
Electrochemistry
Energy Storage

Background:

Aqueous zinc-ion batteries (ZIBs) are promising for large-scale energy storage due to safety, cost, and environmental benefits.
However, Zn anode issues like dendrites, corrosion, and hydrogen evolution limit ZIB lifespan and practical application.
Two-dimensional (2D) materials are explored as advanced Zn anodes to overcome these limitations.

Purpose of the Study:

To review and guide the rational design of 2D materials for stable Zn anodes in ZIBs.
To combine fundamental principles with research progress for practical ZIB applications.
To propose future development perspectives for advanced Zn anodes.

Main Methods:

Introduction to the fundamental principles of 2D materials in mitigating Zn anode drawbacks.

Keywords:

2D materials Large-scale energy storage application Lifespan Zinc-ion battery Zn anode

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Comprehensive summary of designed strategies using typical 2D materials for stable Zn anodes.

Analysis of the unique properties of 2D materials for ZIB anode engineering.

Main Results:

2D materials possess atomic thickness, high surface area, active sites, mechanical strength, and unique electrical properties beneficial for Zn anodes.
Engineered 2D materials effectively address Zn dendrite formation, corrosion, and hydrogen evolution.
Designed strategies for various 2D materials demonstrate their potential for stable ZIB anodes.

Conclusions:

2D materials are a promising alternative for developing stable and high-performance Zn anodes in ZIBs.
Rational design strategies leveraging 2D material properties are crucial for practical ZIB applications.
Further development of advanced Zn anodes using 2D materials holds significant potential for future energy storage solutions.