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Complex-tensor theory of simple smectics.

Jack Paget1, Marco G Mazza1,2, Andrew J Archer1

  • 1Interdisciplinary Centre for Mathematical Modelling and Department of Mathematical Sciences, Loughborough University, Loughborough, Leicestershire, LE11 3TU, UK.

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|February 24, 2023
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Summary
This summary is machine-generated.

This study introduces a new tensor order parameter for modeling lamellar smectic materials. This advanced approach simplifies complex simulations of these fluid-solid states, aiding in understanding their unique properties.

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Area of Science:

  • Soft Matter Physics
  • Materials Science
  • Continuum Mechanics

Background:

  • Lamellar materials, like smectics, exhibit unique properties due to layered self-assembly.
  • Smectics, existing between fluid and solid states, are challenging to model, especially in confined spaces.
  • Existing models struggle with the orientational and positional ordering characteristic of smectics.

Purpose of the Study:

  • To develop a novel theoretical framework for describing simple lamellar smectics.
  • To introduce a complex tensor order parameter capturing local ordering, layer displacement, and orientation.
  • To enable the simulation of complex mesoscopic structures in smectic systems.

Main Methods:

  • Proposed a complex tensor order parameter for describing lamellar smectics.
  • Incorporated regularization of singularities within defect cores to handle dislocations and disclinations continuously.
  • Developed a theory that simplifies numerical analysis for mesoscopic studies.

Main Results:

  • The proposed tensor theory successfully describes local lamellar ordering, layer displacement, and orientation.
  • The theory continuously accounts for dislocations and disclinations by regularizing defect core singularities.
  • Enabled simulation of arrested configurations and inclusion-induced local ordering.

Conclusions:

  • The tensorial theory provides a simplified and continuous mathematical description for simple smectics.
  • This advancement facilitates the study of mesoscopic structures in topologically complex lamellar systems.
  • The new model aids in understanding the functional properties of self-assembling layered materials.