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Valence Bond Theory02:42

Valence Bond Theory

Coordination compounds and complexes exhibit different colors, geometries, and magnetic behavior, depending on the metal atom/ion and ligands from which they are composed. In an attempt to explain the bonding and structure of coordination complexes, Linus Pauling proposed the valence bond theory, or VBT, using the concepts of hybridization and the overlapping of the atomic orbitals. According to VBT, the central metal atom or ion (Lewis acid) hybridizes to provide empty orbitals of suitable...

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Spin pumping through nanocrystalline topological insulators.

David M Burn1, Jheng-Cyuan Lin2, Ryuji Fujita2

  • 1Diamond Light Source, Harwell Science and Innovation Campus, Didcot, Oxfordshire OX11 0DE, United Kingdom.

Nanotechnology
|March 22, 2023
PubMed
Summary
This summary is machine-generated.

Nanocrystalline topological insulators (TIs) enhance spin pumping for spintronic devices. This study demonstrates efficient spin current transfer through TIs using x-ray ferromagnetic resonance, overcoming limitations of single-crystalline films.

Keywords:
ferromagnetic resonancenanocrystalline quantum materialsspin pumpingtopological insulatorsx-ray magnetic circular dichroism

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Area of Science:

  • Condensed Matter Physics
  • Materials Science
  • Spintronics

Background:

  • Topological surface states (TSSs) in topological insulators (TIs) enable dissipationless spin transport.
  • Conventional spintronic devices like spin valves use trilayer structures with ferromagnetic (FM) and non-magnetic layers.
  • Single-crystalline TIs have limited spin pumping efficiency due to a single spin-momentum locked channel.

Purpose of the Study:

  • To investigate the potential of nanocrystalline TI films for enhanced spin pumping.
  • To demonstrate efficient spin current transfer through TI layers in a FM/TI/FM heterostructure.

Main Methods:

  • Fabrication of nanocrystalline TI films with grain sizes preventing TSS hybridization.
  • Utilized element-selective, x-ray based ferromagnetic resonance (XFMR) spectroscopy.
  • Measured spin pumping from a FM layer, through the TI layer, and into a second FM layer (spin sink).

Main Results:

  • Demonstrated successful spin pumping from a ferromagnetic layer through a topological insulator.
  • Showcased efficient spin current transfer into a second ferromagnetic layer acting as a spin sink.
  • Nanocrystalline TI films provide multiple spin channels, enhancing spin pumping efficiency compared to single-crystalline films.

Conclusions:

  • Nanocrystalline TI films are promising for improving spin current generation and transfer in spintronic devices.
  • The study validates the use of XFMR for probing spin dynamics in TI-based heterostructures.
  • This approach offers a pathway to more efficient spintronic devices by leveraging the unique properties of TIs.