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Updated: Aug 2, 2025

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Spectral and Angle-Resolved Magneto-Optical Characterization of Photonic Nanostructures
Published on: November 21, 2019
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Ultrafast light-driven magneto-optical nonlinearity in ferromagnetic heterostructures
Optics Letters
|April 14, 2023
Summary
Ultrafast laser pulses dynamically control magnetization in metallic heterostructures. This study reveals terahertz radiation generation mechanisms, highlighting spin-to-charge conversion and demagnetization as key factors.
Area of Science:
- Condensed Matter Physics
- Materials Science
- Optoelectronics
Background:
- Dynamic control of magnetization using short laser pulses is a growing research area.
- Previous studies explored transient magnetization via second-harmonic generation and time-resolved magneto-optical effects.
- The ultrafast light-driven magneto-optical nonlinearity in ferromagnetic heterostructures for terahertz (THz) radiation requires further clarification.
Purpose of the Study:
- To investigate THz generation from a metallic heterostructure (Pt/CoFeB/Ta).
- To elucidate the underlying physical mechanisms contributing to THz emission.
- To establish THz-emission spectroscopy as a tool for studying picosecond-timescale nonlinear magneto-optical effects.
Main Methods:
- Fabrication of a Pt/CoFeB/Ta metallic heterostructure.
- Utilizing THz-emission spectroscopy to probe ultrafast dynamics.
- Analyzing contributions from magnetization-induced optical rectification, spin-to-charge current conversion, and ultrafast demagnetization.
Main Results:
- Observed THz generation from the Pt/CoFeB/Ta heterostructure.
- Quantified the contributions to THz generation: ~6-8% from magnetization-induced optical rectification.
- ~94-92% from spin-to-charge current conversion and ultrafast demagnetization.
Conclusions:
- Spin-to-charge current conversion and ultrafast demagnetization are dominant mechanisms for THz generation in this heterostructure.
- THz-emission spectroscopy is demonstrated as an effective technique for probing picosecond-timescale nonlinear magneto-optical phenomena.
- The findings advance understanding of light-matter interactions in magnetic heterostructures for THz applications.
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