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Related Concept Videos

Photoluminescence: Applications01:14

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Photoluminescence offers a wide range of applications due to its inherent sensitivity and selectivity. This technique allows for both direct and indirect analyses of the analyte. Direct quantitative analysis is possible when the analyte exhibits a favorable quantum yield for fluorescence or phosphorescence. However, an indirect analysis may be feasible if the analyte is not fluorescent or phosphorescent, or if the quantum yield is unfavorable. Indirect methods include reacting the analyte with...
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Related Experiment Video

Updated: Aug 1, 2025

Determination of the Excitation and Coupling Rates Between Light Emitters and Surface Plasmon Polaritons
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Experimental characterization techniques for plasmon-assisted chemistry.

Emiliano Cortés1, Roland Grzeschik2, Stefan A Maier3,4

  • 1Chair in Hybrid Nanosystems, Nano-Institute Munich, Faculty of Physics, Ludwig-Maximilians-Universität München, München, Germany. emiliano.cortes@lmu.de.

Nature Reviews. Chemistry
|April 28, 2023
PubMed
Summary
This summary is machine-generated.

Understanding plasmon-assisted chemistry requires advanced techniques to analyze nanoscale interactions. This review details experimental methods for characterizing optical fields, heat, and charge transfer dynamics for better scientific insight.

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Area of Science:

  • Nanoscale science and engineering
  • Physical chemistry
  • Materials science

Background:

  • Plasmon-assisted chemistry involves complex nanoscale interactions: electromagnetic fields, heat, and charge transfer.
  • Disentangling the roles of these factors is challenging.
  • Characterizing plasmonic/molecular systems requires deep knowledge of their chemical, structural, and spectral properties.

Purpose of the Study:

  • To review experimental techniques for characterizing plasmon-assisted chemistry.
  • To address challenges in resolving nanoscale phenomena.
  • To discuss the transition from ensemble to single-particle measurements.

Main Methods:

  • Focus on experimental techniques for detailed characterization.
  • Utilize time-resolved methods to monitor dynamics across femtosecond to millisecond timescales.
  • Employ techniques with spatial, energetic, and temporal resolution for optical near fields, temperature, and hot carriers.

Main Results:

  • Experimental techniques are crucial for disentangling the interplay of electromagnetic fields, heat, and charge transfer.
  • Time-resolved measurements are essential due to the wide range of process timescales.
  • Characterization requires high spatial, energetic, and temporal resolution.

Conclusions:

  • A comprehensive understanding of plasmon-assisted chemistry necessitates advanced experimental techniques.
  • Bridging ensemble and single-particle measurements presents significant challenges.
  • Joint experimental and theoretical efforts are vital for advancing the field.