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Ultrafast terahertz emission from emerging symmetry-broken materials
Jacob Pettine1, Prashant Padmanabhan1, Nicholas Sirica1
1Center for Integrated Nanotechnologies, Los Alamos National Laboratory, Los Alamos, NM, 87545, USA.
Light, Science & Applications
|May 31, 2023
Summary
Terahertz emission spectroscopy reveals material properties by analyzing broken symmetries. This technique probes ultrafast dynamics in emerging materials and nanoscale systems for advanced applications.
Area of Science:
- Condensed matter physics
- Materials science
- Optics
Background:
- Nonlinear optical spectroscopies are essential for studying material properties and light-induced dynamics.
- Terahertz (THz) emission spectroscopy directly tracks ultrafast evolution in materials and interfaces.
- Analyzing THz emission often involves complex mechanistic models of polarization, magnetization, and charge currents.
Purpose of the Study:
- To frame THz emission spectroscopy through the lens of fundamental symmetry principles.
- To generalize the understanding of nonlinear optical responses across diverse material systems.
- To explore the application of THz emission spectroscopy in emerging and low-dimensional materials.
Main Methods:
- Utilizing symmetry considerations (spatial, temporal, point group) to interpret THz emission.
- Reviewing recent studies on strongly correlated, magnetic, multiferroic, and topological systems.
- Investigating nanoscale structuring and its impact on THz emission properties.
Main Results:
- Symmetry principles provide a generalized framework for understanding THz emission.
- THz emission spectroscopy successfully probes the fundamental properties of various advanced materials.
- Nanoscale engineering of material symmetries enhances THz emission for probing ultrafast phenomena.
Conclusions:
- Symmetry is a key factor in enabling and controlling THz emission.
- THz emission spectroscopy is a powerful tool for investigating novel materials and nanoscale physics.
- Interplay of symmetries and hybrid structures can lead to the discovery of new phenomena.

