Electrical detection of spin pumping in van der Waals ferromagnetic Cr₂Ge₂Te₆ with low magnetic damping

The discovery of magnetic order in atomically-thin van der Waals materials has strengthened the alliance between spintronics and two-dimensional materials. An important use of magnetic two-dimensional materials in spintronic devices, which has not yet been demonstrated, would be for coherent spin injection via the spin-pumping effect. Here, we report spin pumping from Cr₂Ge₂Te₆ into Pt or W and detection of the spin current by inverse spin Hall effect. The magnetization dynamics of the hybrid Cr₂Ge₂Te₆/Pt system are measured, and a magnetic damping constant of ~ 4-10 × 10^-4 is obtained for thick Cr₂Ge₂Te₆ flakes, a record low for ferromagnetic van der Waals materials. Moreover, a high interface spin transmission efficiency (a spin mixing conductance of 2.4 × 10¹⁹/m²) is directly extracted, which is instrumental in delivering spin-related quantities such as spin angular momentum and spin-orbit torque across an interface of the van der Waals system. The low magnetic damping that promotes efficient spin current generation together with high interfacial spin transmission efficiency suggests promising applications for integrating Cr₂Ge₂Te₆ into low-temperature two-dimensional spintronic devices as the source of coherent spin or magnon current.