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Electric-Field-Driven Spin Resonance by On-Surface Exchange Coupling to a Single-Atom Magnet
Soo-Hyon Phark1,2,3, Hong Thi Bui1,2, Alejandro Ferrón4
1Center for Quantum Nanoscience, Institute for Basic Science (IBS), Seoul, 03760, Republic of Korea.
Researchers demonstrate coherent control of individual spins on surfaces using a novel electron spin resonance (ESR) technique. This method enables addressing and controlling spins without direct tip interaction, paving the way for multi-qubit systems.
Area of Science:
- Quantum physics
- Surface science
- Materials science
Background:
- Coherent control of individual spins on surfaces is crucial for quantum technologies.
- Electron spin resonance (ESR) in scanning tunneling microscopy (STM) has enabled spin manipulation.
- Developing new methods for addressing and controlling multiple spins is an ongoing challenge.
Purpose of the Study:
- To investigate the electron spin resonance (ESR) of a single hydrogenated Ti atom exchange-coupled to a Fe adatom on a surface.
- To demonstrate a new ESR scheme for coherent control of individual spins without direct tip interaction.
- To establish a feasible implementation of spin-based multi-qubit systems on surfaces.
Main Methods:
- Combined experimental and theoretical modeling of ESR using STM.
- Atom manipulation to position a Fe adatom near a hydrogenated Ti atom.
- Continuous wave and pulsed ESR measurements to analyze Rabi rates and spin interactions.
Main Results:
- The ESR of the Ti spin showed two contributions: one from the STM tip and another from the exchange-coupled Fe adatom.
- The Fe contribution to the spin interaction was comparable to the tip's and tunable with a magnetic field.
- The new ESR scheme successfully addressed and coherently controlled individual spins without direct tip magnetic interaction.
Conclusions:
- A novel ESR scheme enables coherent control of individual spins on surfaces.
- This method allows for addressing spins without relying on magnetic interaction with the STM tip.
- The study presents a viable approach for building spin-based multi-qubit systems on surfaces.
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