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Nickel hydroxide-decorating potassium-doped graphitic carbon nitride for boosting photocatalytic carbon dioxide
Mianmian Zhai1, Yu Zhang1, Jixiang Xu1
1Key Laboratory of Eco-chemical Engineering, Taishan Scholar Advantage and Characteristic Discipline Team of Eco-Chemical Process and Technology, Qingdao University of Science and Technology, Qingdao 266042, China; College of Chemistry and Molecular Engineering, Qingdao University of Science and Technology, Qingdao 266042, China.
Abstract:
In this study, nickel hydroxide (Ni(OH)2) was employed to modify potassium (K)-doped graphitic carbon nitride (g-C3N4, CN) for enhancing photocatalytic CO2 reduction. The light absorption and charge separation performances of CN were enhanced after modification. Experiments and theoretical calculations indicated that the loaded Ni(OH)2 could gather electrons, facilitate adsorption and activation of CO2. The optimized photocatalyst exhibited high CO2 reductive rate with CO and CH4 yields of 42.6 and 3.5 μmol g-1, respectively after 3 h irradiation in the presence of 0.5 mL water, which was 1.4 and 4.6 times higher than the yields on K-doped CN and Ni(OH)2-decorated CN, respectively. This work provides new thought for enhancing CO2 reductive performance of CN.
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