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SO-modified porous carbon as a highly active electrocatalyst for efficient H2O2 generation
Kunhong Jiang1, Zhenyu Li1,2, Ying Yu1
1College of Chemistry and Chemical Engineering, Inner Mongolia Engineering and Technology Research Center for Catalytic Conversion and Utilization of Carbon Resource Molecules, Inner Mongolia University, Hohhot 010021, China. weihang@imu.edu.cn.
Abstract:
A SO-decorated porous carbon electrocatalyst that exhibits excellent 2e- oxygen reduction reaction activity is synthesized using UV-curing technology in combination with a pyrolysis process. The H2O2 selectivity using the SO-porous C shows 95.1% at 0.4 V and delivers a H2O2 production rate of 604.2 mmol gcat-1 h-1. Density-functional theory calculations reveal the reasons for the improvement of catalytic performance.
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