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Updated: Jul 19, 2025

Cooling Rate Dependent Ellipsometry Measurements to Determine the Dynamics of Thin Glassy Films
Published on: January 26, 2016
Dynamical heterogeneity in active glasses is inherently different from its equilibrium behavior
Kallol Paul1, Anoop Mutneja1, Saroj Kumar Nandi1
1Tata Institute of Fundamental Research Center for Interdisciplinary Science, Hyderabad 500046, Telangana, India.
Active glasses, unlike equilibrium glasses, exhibit complex dynamic heterogeneity. This study combines simulations and mode-coupling theory to reveal significant differences in their glassy dynamics.
Area of Science:
- Physics
- Soft Matter Physics
- Non-equilibrium Systems
Background:
- Activity-driven glassy dynamics are observed in various systems like cell migration and colony behavior.
- Active glasses were previously thought to resemble equilibrium glasses at an effective temperature.
- The physics of glass transition remains a complex and actively researched area.
Purpose of the Study:
- To investigate the fundamental differences between active and equilibrium glasses.
- To analyze the impact of activity on dynamic heterogeneity in glassy systems.
- To develop and validate theoretical models for active glassy dynamics.
Main Methods:
- Large-scale computer simulations were employed to model active glassy systems.
- Analytical mode-coupling theory (MCT) was extended for active systems.
- Four distinct methods were used to reliably estimate dynamic heterogeneity length scales.
Main Results:
- Active glasses are fundamentally different from equilibrium glasses, contrary to prior assumptions.
- While relaxation dynamics can appear equilibrium-like, activity significantly alters dynamic heterogeneity.
- Dramatic growth in dynamic heterogeneity was observed in active glasses, with varying scales for similar relaxation times.
Conclusions:
- The study reveals non-trivial effects of activity on dynamic heterogeneity, challenging previous assumptions.
- Extended active MCT provides good qualitative agreement with simulation results for dynamic heterogeneity.
- Findings offer new insights into the role of dynamic heterogeneity in glassy dynamics, with potential implications for equilibrium systems.
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