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  2. Mixed-dimensional Van Der Waals Heterostructures For Boosting Electricity Generation.
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Mixed-Dimensional van der Waals Heterostructures for Boosting Electricity Generation.

Haoran Kong1,2, Huiying Yao3, Yuting Li1,2

  • 1State Key Laboratory of Multiphase Complex Systems, Institute of Process Engineering, Chinese Academy of Sciences, Beijing 100190, P. R. China.

ACS Nano
|September 12, 2023

View abstract on PubMed

Summary
This summary is machine-generated.

This study introduces a novel graphene-based hydrovoltaic device using SiC whiskers for enhanced energy harvesting. The developed device efficiently converts environmental energy and powers a self-sufficient desalination system.

Keywords:
electricity generationelectrophoretic depositiongrapheneintegrated devicesmixed-dimensional van der Waals heterostructuressilicon carbide whiskers

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Area of Science:

  • Materials Science
  • Renewable Energy
  • Nanotechnology

Background:

  • Hydrovoltaic devices offer a promising avenue for renewable energy harvesting, crucial for micro/nano power systems.
  • Graphene-based hydrovoltaic devices with innovative microstructures are trending, but face challenges in fabrication and performance enhancement.
  • Existing methods for improving ion/electron redistribution in graphene hydrovoltaics are complex and offer limited control.

Purpose of the Study:

  • To develop a simplified fabrication process for high-performance graphene-based hydrovoltaic devices.
  • To enhance the output performance of hydrovoltaic devices through novel material integration.
  • To demonstrate a practical application of these devices in a self-powered desalination system.

Main Methods:

  • Utilized electrophoretic deposition (EPD) for SiC whiskers (SiCw)-assisted graphene transfer.
  • Fabricated graphene/SiCw (GS) mesh films with mixed-dimensional van der Waals (vdW) heterostructures.
  • Designed and integrated hydrovoltaic devices into a self-powered desalination-monitoring system.
  • Main Results:

    • Significantly boosted output performance of the graphene/SiCw hydrovoltaic devices.
    • Achieved high graphene integrity and prominent negative surface charge via vdW heterostructures.
    • Successfully demonstrated electricity generation from ionic solutions to power a deionization process.

    Conclusions:

    • The EPD-driven SiCw-assisted graphene transfer simplifies device fabrication and enhances hydrovoltaic performance.
    • The developed graphene/SiCw heterostructures effectively promote ion/electron redistribution for improved energy conversion.
    • Integrated hydrovoltaic devices offer an efficient strategy for sustainable energy harvesting and utilization, exemplified by the desalination system.