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Updated: Jul 15, 2025

Measurement of Scattering Nonlinearities from a Single Plasmonic Nanoparticle

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Published on: January 3, 2016

Nonlinear Plasmonics in Nanostructured Phosphorene.

Line Jelver¹, Joel D Cox^1,2

¹POLIMA─Center for Polariton-driven Light-Matter Interactions, University of Southern Denmark, Campusvej 55, DK-5230 Odense M, Denmark.

|October 4, 2023

Summary

This summary is machine-generated.

Phosphorene nanoribbons support tunable plasmons for optoelectronics. These localized plasmons trigger intense nonlinear optical responses, making nanostructured phosphorene a promising material for advanced photonic applications.

Keywords:

nanophotonics nanoribbons nonlinear optics phosphorene plasmons quantum plasmonics

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Area of Science:

Materials Science
Condensed Matter Physics
Nanophotonics

Background:

Phosphorene is an atomically thin semiconductor with excellent optical properties.
Electrical doping allows tuning of light-matter interactions in phosphorene.
Plasmon resonances are expected in highly doped phosphorene, exhibiting anisotropy and optical confinement.

Purpose of the Study:

To investigate localized plasmons in phosphorene nanoribbons (PNRs).
To explore the tunability of these plasmons concerning edge termination and doping polarity.
To demonstrate the potential for intense nonlinear optical responses at moderate doping levels.

Main Methods:

Utilized a second-principles theoretical framework.
Employed maximally localized Wannier functions derived from ab initio electronic structure calculations.
Performed atomistic simulations to analyze linear and nonlinear optical responses on mesoscopic scales.

Main Results:

Demonstrated high tunability of localized plasmons in PNRs.
Observed plasmon tunability related to edge termination and doping charge polarity.
Showcased intense nonlinear optical responses, including high-harmonic generation, at moderate doping levels.
Identified synergy between electronic band structure and plasmonic confinement.

Conclusions:

Nanostructured phosphorene supports highly tunable localized plasmons.
PNRs exhibit significant nonlinear optical properties, particularly high-harmonic generation.
Phosphorene is a versatile candidate for nonlinear plasmonics and advanced optoelectronic devices.