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Nonlinear Plasmonics in Nanostructured Phosphorene.

Line Jelver1, Joel D Cox1,2

  • 1POLIMA─Center for Polariton-driven Light-Matter Interactions, University of Southern Denmark, Campusvej 55, DK-5230 Odense M, Denmark.

ACS Nano
|October 4, 2023
PubMed
Summary
This summary is machine-generated.

Phosphorene nanoribbons support tunable plasmons for optoelectronics. These localized plasmons trigger intense nonlinear optical responses, making nanostructured phosphorene a promising material for advanced photonic applications.

Keywords:
nanophotonicsnanoribbonsnonlinear opticsphosphoreneplasmonsquantum plasmonics

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Area of Science:

  • Materials Science
  • Condensed Matter Physics
  • Nanophotonics

Background:

  • Phosphorene is an atomically thin semiconductor with excellent optical properties.
  • Electrical doping allows tuning of light-matter interactions in phosphorene.
  • Plasmon resonances are expected in highly doped phosphorene, exhibiting anisotropy and optical confinement.

Purpose of the Study:

  • To investigate localized plasmons in phosphorene nanoribbons (PNRs).
  • To explore the tunability of these plasmons concerning edge termination and doping polarity.
  • To demonstrate the potential for intense nonlinear optical responses at moderate doping levels.

Main Methods:

  • Utilized a second-principles theoretical framework.
  • Employed maximally localized Wannier functions derived from ab initio electronic structure calculations.
  • Performed atomistic simulations to analyze linear and nonlinear optical responses on mesoscopic scales.

Main Results:

  • Demonstrated high tunability of localized plasmons in PNRs.
  • Observed plasmon tunability related to edge termination and doping charge polarity.
  • Showcased intense nonlinear optical responses, including high-harmonic generation, at moderate doping levels.
  • Identified synergy between electronic band structure and plasmonic confinement.

Conclusions:

  • Nanostructured phosphorene supports highly tunable localized plasmons.
  • PNRs exhibit significant nonlinear optical properties, particularly high-harmonic generation.
  • Phosphorene is a versatile candidate for nonlinear plasmonics and advanced optoelectronic devices.