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Updated: Jul 12, 2025
Synthesis and Performance Characterizations of Transition Metal Single Atom Catalyst for Electrochemical CO2 Reduction
Published on: April 10, 2018
Facile synthesis of supported CuNi nano-clusters as an electrochemical CO2 reduction catalyst with broad potential
Jiale Wang1, Fan Li1, Runhua Li1
1State Key Laboratory of Metal Matrix Composites, School of Materials Science and Engineering, Shanghai Jiao Tong University, Shanghai 200240, China. jianbowu@sjtu.edu.cn.
Abstract:
A nitrogen-doped carbon-supported CuNi bimetallic nanocluster catalyst (CuNi-NC) was first synthesized via a facile ZIF-derived method. With a synergistic effect between Cu and Ni, the catalyst exhibited a maximum FECO of 96.3%. FECO is higher than 90% in a broad potential range of 600 mV, which was ascribed to the controllable pore size distribution. Density functional theory further demonstrated the preferred formation of *COOH in the catalytic process.
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