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Updated: Aug 6, 2026

Direct Imaging of Laser-driven Ultrafast Molecular Rotation
Published on: February 4, 2017
Tunable four-wave mixing enabled by a self-phase modulation of chirped pulses
Abstract:
We experimentally demonstrate how a concatenation of the standard and microstructure fiber segments permits adjusting the four-wave mixing sideband position over a large spectral range by varying the chirp of an input pulsed pump at a fixed wavelength in the presence of a self-phase modulation. The blue- and redshifted sidebands can stand aside over ∼200 nm and ∼450 nm from the pump, respectively, which agrees well with the numerical simulations. We validate our approach by showing the feasibility of CARS imaging.
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