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Active Solid-State Nanopores: Self-Driven Flows/Chaos at the Liquid-Gas Nanofluidic Interface
Vinitha Johny1,2,3, Siddharth Ghosh1,2,3,4,5
1International Center for Nanodevices, INCeNSE-TBI, Indian Institute of Science Campus, Bangalore 560 012, Karnataka, India.
Langmuir : the ACS Journal of Surfaces and Colloids
|November 29, 2023
Summary
We discovered self-driven fluid flow in nanoscale pores, leading to chaotic motion and a novel "active solid-state nanopore" concept for switching flow states. This advances understanding of fluid dynamics and enables new applications.
Area of Science:
- Nanofluidics
- Fluid Dynamics
- Interface Phenomena
Background:
- Investigating fluid behavior at the nanoscale is crucial for developing advanced technologies.
- Understanding liquid-gas interfaces in confined spaces presents unique challenges.
- External forces are typically required to drive flow in micro/nanofluidic systems.
Purpose of the Study:
- To comprehensively study self-driven flow dynamics at the liquid-gas interface in nanofluidic pores without external forces.
- To analyze Rayleigh-Taylor instability phenomena in sub-100 nm pores.
- To introduce and explore the concept of an
- active solid-state nanopore
- with self-driven flow switching capabilities.
Main Methods:
- Theoretical modeling to derive a flow velocity equation.
- Computational simulations for validation and analysis of mass transfer efficiency.
- Experimental observation of nanoscale chaotic fluid motion.
Main Results:
- A validated flow velocity equation for self-driven nanofluidic systems.
- Demonstration of self-driven flow switching in an
- active solid-state nanopore
- without mechanical parts.
- Observation of nanoscale chaos in fluid dynamics, distinct from macroscopic turbulence.
Conclusions:
- Self-driven nanofluidics offers a new paradigm for fluid control at the liquid-gas interface.
- The
- active solid-state nanopore
- concept has potential for applications in sensing, healthcare, and energy.
- This research bridges the understanding of classical and quantum fluid dynamics in confined environments.

