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Perspective on Tailored Nanostructure-Dominated SPP Effects for SERS.

Haifeng Hu1, Yi Tian1, Peipei Chen1,2

  • 1Nanofabrication Laboratory, National Center for Nanoscience and Technology, Beijing, 100190, China.

Advanced Materials (Deerfield Beach, Fla.)
|November 30, 2023
PubMed
Summary
This summary is machine-generated.

Surface plasmon polaritons (SPPs) enhance surface-enhanced Raman scattering (SERS) more than localized surface plasmon resonance (LSPR) hot spots. Tailored designs for SPP excitation are crucial for high-performance SERS devices.

Keywords:
coupling of single‐/coupled‐mode SPPs and LSPRin‐/ex situ SERS excitationsquantitative design of SPPs‐manipulated structuresspatiotemporally separable SPPs multiple processesstate‐of‐the‐art fabrication

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Area of Science:

  • Plasmonics
  • Nanophotonics
  • Spectroscopy

Background:

  • Localized surface plasmon resonance (LSPR) typically generates strong surface-enhanced Raman scattering (SERS) at nanogaps.
  • Surface plasmon polaritons (SPPs) also excite SERS but are less explored despite their importance in high-performance devices.

Purpose of the Study:

  • To review and comment on SPPs and their coupling with LSPR for SERS.
  • To highlight the role of SPPs in SERS and discuss fabrication approaches.
  • To emphasize quantitative design for high-performance SERS chips.

Main Methods:

  • Review of existing literature on SPPs, LSPR, and SERS.
  • Analysis of plasmonic/dielectric structures and configurations for SPP generation.
  • Discussion of fabrication approaches for SERS devices.

Main Results:

  • SPPs offer an alternative and potentially more effective mechanism for SERS excitation compared to LSPR hot spots.
  • Coupling between SPPs and LSPR can be tuned for optimized SERS performance.
  • Quantitative design of SPP-based configurations is key for advanced SERS applications.

Conclusions:

  • SPPs are critical for high-performance SERS, warranting further attention.
  • Tailored structures dominating SPP effects, coupled with LSPR, pave the way for innovative SERS devices.
  • Focus on quantitative design and batch manufacturability is essential for practical SERS applications.