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Constructing a Highly Robust Interface Film for Enhancing Rate Performance of Graphite Anode via a Novel Electrolyte

Qiurong Chen1, Min Chen2,3, Zhangyating Xie1

  • 1School of Chemistry, South China Normal University, Guangzhou 510006, Guangdong, China.

The Journal of Physical Chemistry Letters
|November 30, 2023
PubMed
Summary

A novel electrolyte additive, FTMS, enhances lithium-ion battery performance by creating a robust solid electrolyte interphase (SEI) on graphite anodes, improving capacity retention and rate capability.

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Battery Technology

Background:

  • The solid electrolyte interphase (SEI) is crucial for high power output in Lithium-ion batteries (LIBs).
  • Graphite anodes in LIBs often suffer from slow lithium insertion/desertion kinetics, limiting performance.

Purpose of the Study:

  • To enhance the rate performance of graphite anodes in LIBs.
  • To develop a robust and stable SEI using a novel electrolyte additive.

Main Methods:

  • Modification of electrolyte with 1H,1H,2H,2H-perfluorooctyltrimethoxysilane (FTMS).
  • Experimental characterizations and theoretical calculations to analyze SEI formation and properties.

Main Results:

  • Addition of 2% FTMS improved capacity retention from 77.6% to 91.2% at 0.5 C after 100 cycles.
  • Capacity at 2 C increased significantly from 86 to 229 mAh g⁻¹ with FTMS.
  • FTMS formed a flexible and conductive SEI layer composed of fluoride-containing organic lithium salt and silicon-containing polymer.

Conclusions:

  • FTMS is an effective additive for constructing a robust and stable SEI on graphite anodes.
  • The modified SEI enhances lithium ion kinetics, leading to improved LIB performance.
  • This approach offers a viable solution for overcoming the kinetic limitations of graphite anodes in LIBs.