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Crystal Growth: Principles of Crystallization01:25

Crystal Growth: Principles of Crystallization

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Crystallization is a phase transformation process in which crystals are precipitated from a supersaturated solution or formed from other sources. During crystallization, atoms or molecules arrange themselves into a well-defined, rigid crystal lattice to minimize energy.
Initiating crystallization involves manipulating the concentration of the solute and the temperature of the solution. Since crystal growth occurs when the ratio of concentration and solubility of the solute in the solvent...
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Methods of Ex Situ and In Situ Investigations of Structural Transformations: The Case of Crystallization of Metallic Glasses
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Boosting Energy Storage Performance of Glass Ceramics via Modulating Defect Formation During Crystallization.

Fei Shang1, Juwen Wei1, Jiwen Xu1

  • 1Electronical Information Materials and Devices Engineering Research Center of Ministry of Education, Guangxi Key Laboratory of Information Materials, and School of Material Science and Engineering, Guilin University of Electronic Technology, Guilin, 541004, China.

Advanced Science (Weinheim, Baden-Wurttemberg, Germany)
|December 8, 2023
PubMed
Summary
This summary is machine-generated.

Researchers developed advanced BaTiO3-based glass ceramics for high-energy storage devices. These materials achieve ultrahigh recoverable energy storage density (Wrec) and discharge energy storage density (Wd) with excellent efficiency and power density.

Keywords:
defect modulationdielectric energy storageglass ceramicspower densitytwin structure

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Area of Science:

  • Materials Science
  • Solid State Physics
  • Dielectric Materials

Background:

  • Miniaturization of high-power devices necessitates materials with superior energy storage capabilities.
  • Achieving high recoverable energy storage density (Wrec) and discharge energy storage density (Wd) simultaneously with high efficiency (η) and power density (Pd) in dielectrics is challenging.
  • Glass ceramics currently lag behind other dielectric materials in energy storage performance.

Purpose of the Study:

  • To develop advanced BaTiO3-based glass ceramics with enhanced dielectric energy storage properties.
  • To investigate the impact of microstructure on energy storage performance.
  • To demonstrate the potential of glass ceramics for high and pulsed power applications.

Main Methods:

  • A strategy of defect formation modulation was employed.
  • An "amorphous-disordered-ordered" microstructure was engineered in BaTiO3-based glass ceramics.
  • Key energy storage parameters (Wrec, η, Wd, Pd) were measured.

Main Results:

  • The engineered glass ceramics achieved an ultrahigh recoverable energy storage density (Wrec) of 12.04 J cm⁻³.
  • A high energy storage efficiency (η) of 81.1% was recorded.
  • An ultrahigh discharge energy storage density (Wd) of 11.98 J cm⁻³ was obtained with a superb power density (Pd) of 973 MW cm⁻³.

Conclusions:

  • The defect formation modulation strategy successfully created an "amorphous-disordered-ordered" microstructure, significantly boosting energy storage performance.
  • The developed BaTiO3-based glass ceramics exhibit outstanding energy storage capabilities, surpassing current limitations.
  • These findings highlight the immense potential of glass ceramics for next-generation high and pulsed power applications.