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Synthesis and Performance Characterizations of Transition Metal Single Atom Catalyst for Electrochemical CO2 Reduction

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Recent Progress on Perovskite-Based Electrocatalysts for Efficient CO₂ Reduction.

Tong Wu¹, Lihua Zhang¹, Yinbo Zhan¹

¹Low Carbon College, Shanghai Jiaotong University, Shanghai 201306, China.

Molecules (Basel, Switzerland)

|December 23, 2023

Summary

This review covers inorganic perovskite materials for efficient carbon dioxide reduction (CO2RR) catalysis. These materials offer tunable properties for converting CO2 into valuable products, aiding carbon neutrality goals.

Keywords:

C1 and C2+ products CO2 electroreduction reaction perovskite structural evolution synthesis

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Area of Science:

Materials Science
Electrochemistry
Catalysis

Background:

Efficient carbon dioxide reduction reaction (CO2RR) is crucial for carbon neutrality, requiring effective and low-cost catalysts.
Inorganic perovskite-based materials show promise for electrochemical CO2RR due to their tunable chemical compositions and advanced catalytic performance.

Purpose of the Study:

To systematically review the progress of inorganic perovskites and their derivatives in electrochemical CO2RR.
To emphasize the structural evolution and product selectivity of these electrocatalysts.
To propose current challenges and future directions for perovskite-based materials in CO2RR.

Main Methods:

Comprehensive literature review of inorganic perovskites for electrochemical CO2RR.
Analysis of physicochemical characteristics, fabrication methods, and applications.
Focus on structure-property relationships and product selectivity.

Main Results:

Inorganic perovskites exhibit significant potential as electrocatalysts for CO2RR.
Tunable properties of perovskites allow for optimization of catalytic performance and product selectivity.
Review highlights key advancements and areas for further investigation.

Conclusions:

Inorganic perovskites are promising candidates for efficient and cost-effective CO2RR catalysts.
Further research into structural evolution and fabrication methods can enhance catalyst performance.
Addressing current challenges will accelerate the development of perovskite-based CO2RR technologies for carbon neutrality.