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An ionic compound is stable because of the electrostatic attraction between its positive and negative ions. The lattice energy of a compound is a measure of the strength of this attraction. The lattice energy (ΔHlattice) of an ionic compound is defined as the energy required to separate one mole of the solid into its component gaseous ions. For the ionic solid sodium chloride, the lattice energy is the enthalpy change of the process:
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Solid Interfaces for the Garnet Electrolytes.

Wuliang Feng1,2, Yufeng Zhao2, Yongyao Xia1

  • 1Department of Chemistry, Shanghai Key Laboratory of Molecular Catalysis and Innovative Materials, Fudan University, Shanghai, 200433, China.

Advanced Materials (Deerfield Beach, Fla.)
|January 12, 2024
PubMed
Summary
This summary is machine-generated.

Garnet solid-state electrolytes (SSEs) offer high performance for solid-state lithium batteries (SSLBs). This study addresses interfacial challenges like dendrite growth and contact issues, proposing stabilization strategies for improved battery safety and efficiency.

Keywords:
garnetinterfacelithium dendritesolid‐statestability

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Energy Storage

Background:

  • Solid-state electrolytes (SSEs) are crucial for high-energy-density and safe secondary batteries.
  • Garnet-type SSEs show promise for solid-state lithium batteries (SSLBs) due to high ionic conductivity and low reduction potential.
  • Challenges include poor interfacial contact and lithium dendrite growth caused by garnet's elastic modulus and electronic conduction.

Purpose of the Study:

  • To review recent advancements in solid interfaces for garnet electrolytes in SSLBs.
  • To present strategies for suppressing lithium dendrite growth and stabilizing interfaces.
  • To offer insights into the practical application and future development of garnet-based SSLBs.

Main Methods:

  • Review of recent literature on garnet-based solid-state electrolytes.
  • Analysis of interfacial stabilization strategies, including chemical, electrochemical, and mechanical approaches.
  • Discussion of lithium dendrite suppression techniques and interphase design.

Main Results:

  • Garnet SSEs face interfacial challenges impacting SSLB performance and safety.
  • Effective strategies for interfacial stabilization and lithium dendrite suppression have been developed.
  • A novel perspective on interfacial lithiophobia is introduced.

Conclusions:

  • Optimizing solid interfaces is key to unlocking the full potential of garnet-based SSLBs.
  • This work provides a comprehensive understanding of interfacial stabilization for SSEs.
  • Advancements in garnet electrolytes are crucial for the future of the SSLB industry.