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Related Concept Videos

Metallic Solids02:37

Metallic Solids

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Metallic solids such as crystals of copper, aluminum, and iron are formed by metal atoms. The structure of metallic crystals is often described as a uniform distribution of atomic nuclei within a “sea” of delocalized electrons. The atoms within such a metallic solid are held together by a unique force known as metallic bonding that gives rise to many useful and varied bulk properties.
All metallic solids exhibit high thermal and electrical conductivity, metallic luster, and malleability....
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Ionic Crystal Structures02:42

Ionic Crystal Structures

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Ionic crystals consist of two or more different kinds of ions that usually have different sizes. The packing of these ions into a crystal structure is more complex than the packing of metal atoms that are the same size.
Most monatomic ions behave as charged spheres, and their attraction for ions of opposite charge is the same in every direction. Consequently, stable structures for ionic compounds result (1) when ions of one charge are surrounded by as many ions as possible of the opposite...
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Molecular and Ionic Solids02:54

Molecular and Ionic Solids

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Crystalline solids are divided into four types: molecular, ionic, metallic, and covalent network based on the type of constituent units and their interparticle interactions.
Molecular Solids
Molecular crystalline solids, such as ice, sucrose (table sugar), and iodine, are solids that are composed of neutral molecules as their constituent units. These molecules are held together by weak intermolecular forces such as London dispersion forces, dipole-dipole interactions, or hydrogen bonds, which...
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Ionic Compounds: Formulas and Nomenclature03:34

Ionic Compounds: Formulas and Nomenclature

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An element composed of atoms that readily lose electrons (a metal) can react with an element composed of atoms that readily gain electrons (a nonmetal) to produce ions through complete electron transfer. The compound formed by this transfer is stabilized by the electrostatic attractions (ionic bonds) between the oppositely charged ions.
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Voltaic/Galvanic Cells02:47

Voltaic/Galvanic Cells

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Spontaneous Chemical Reactions
Spontaneous redox reactions occur abundantly in nature. The chemical reaction occurring in a disposable AA battery powering our remote controls is one such example of a spontaneous redox reaction. Another example is the immersion of coiled copper wire into an aqueous silver nitrate solution. The reaction shows a gradual, visually impressive color change from colorless to bright blue and the formation of a grey precipitate on the copper wire. In this experiment,...
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Formation of Complex Ions03:45

Formation of Complex Ions

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A type of Lewis acid-base chemistry involves the formation of a complex ion (or a coordination complex) comprising a central atom, typically a transition metal cation, surrounded by ions or molecules called ligands. These ligands can be neutral molecules like H2O or NH3, or ions such as CN− or OH−. Often, the ligands act as Lewis bases, donating a pair of electrons to the central atom. These types of Lewis acid-base reactions are examples of a broad subdiscipline called coordination...
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Synthesis of Ionic Liquid Based Electrolytes, Assembly of Li-ion Batteries, and Measurements of Performance at High Temperature
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Self-assembled hydrated copper coordination compounds as ionic conductors for room temperature solid-state batteries.

Xiao Zhan1, Miao Li1, Xiaolin Zhao2

  • 1State Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, College of Materials, Tan Kah Kee Innovation Laboratory, Collaborative Innovation Center of Chemistry for Energy Materials, Xiamen University, Xiamen, 361005, Fujian, China.

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Summary

Researchers developed novel inorganic-organic hybrid solid-state electrolytes using copper maleate hydrate. These materials exhibit high ionic conductivity and stability for solid-state batteries, offering a promising alternative to current technologies.

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Solid-State Batteries

Background:

  • Current inorganic and polymer solid-state electrolytes face limitations in ionic conductivity, electrode compatibility, and processability.
  • Designing inorganic-organic hybrid electrolytes could synergize the benefits of both material types for improved performance.
  • Metal coordination compounds offer potential as novel solid-state electrolyte materials.

Purpose of the Study:

  • To design and synthesize inorganic-organic hybrid solid-state electrolytes with enhanced ionic conductivity and stability.
  • To explore the potential of metal coordination compounds as room-temperature ionic conductors.
  • To demonstrate the performance of these novel electrolytes in solid-state batteries.

Main Methods:

  • Synthesis of copper maleate hydrate nanoflakes via bottom-up self-assembly.
  • Characterization of the material's structure, including 1D channels, metal nodes, and functional groups.
  • Electrochemical testing to evaluate ionic conductivity, Li+ transference number, and operating voltage window.

Main Results:

  • Copper maleate hydrate exhibits highly-ordered 1D channels facilitating rapid Li+ transport.
  • Achieved ionic conductivity of 1.17 × 10^-4 S cm^-1 at room temperature with a high Li+ transference number of 0.77.
  • Demonstrated a wide operating window of 4.7 V and exceptional compatibility with Li anodes and cathodes, enabling over 800 cycles.

Conclusions:

  • Rational design of metal coordination compounds can yield superior room-temperature ionic conductors.
  • Copper maleate hydrate-based solid-state electrolytes offer a promising pathway for high-performance solid-state batteries.
  • This study provides new insights into exploring metal coordination compounds for advanced energy storage applications.