Recent progress in magnetic polydopamine composites for pollutant removal in wastewater treatment

Various water pollution issues pose a significant threat to human water safety. Magnetic polydopamine composites (MPCs), which can be separated by magnetic fields after the adsorption process, exhibit outstanding adsorption capacity and heterogeneous catalytic properties, making them promising materials for water treatment applications. In particular, by modifying the polydopamine (PDA) coating, MPCs can acquire enhanced high reactivity, antibacterial properties, and biocompatibility. This also provides an attractive platform for further fabrication of hybrid materials with specific adsorption, catalytic, antibacterial, and water-oil separation capabilities. To systematically provide the background knowledge and recent research advances in MPCs, this paper presents a critical review of MPCs for water treatment in terms of both structure and mechanisms of effect in applications. Firstly, the impact of different PDA positions within the composite structure is investigated to summarize the optimization of properties contributed by PDA when acting as the shell, core, or bridge. The roles of various secondary modifications of magnetic materials by PDA in addressing water pollution problems are explored. It is anticipated that this work will be a stimulus for further research and development of magnetic composite materials with real-world application potential.