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Bioinspired Gas Manipulation for Regulating Multiphase Interactions in Electrochemistry.

Zhiyun Long^1,2, Cunming Yu^1,2, Moyuan Cao³

¹Key Laboratory of Bio-inspired Smart Interfacial Science and Technology of Ministry of Education, School of Chemistry, Beihang University, Beijing, 100191, China.

Advanced Materials (Deerfield Beach, Fla.)

|February 22, 2024

Summary

Bioinspired strategies enhance gas manipulation in electrochemical reactions. This review covers advancements in electrode design, mechanisms, and applications like hydrogen evolution and CO2 reduction.

Keywords:

(super)aerophilic electrodes asymmetric electrodes bioinspired electrodes gas bubble manipulation gas consumption reactions gas evolution reactions superaerophobic electrodes

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Area of Science:

Electrochemistry
Materials Science
Bioinspired Engineering

Background:

Gas manipulation is vital for multiphase electrochemical processes.
Nature-inspired strategies offer novel approaches to control gas-liquid interfaces.
Existing methods face challenges in efficiency and selectivity.

Purpose of the Study:

To provide a comprehensive overview of bioinspired gas manipulation in electrochemistry.
To highlight advancements in electrode design and reaction mechanisms.
To summarize applications and future prospects.

Main Methods:

Review of existing literature on bioinspired gas manipulation.
Analysis of superaerophobic, (super)aerophilic, and asymmetric electrode designs.
Categorization of applications in key electrochemical reactions.

Main Results:

Bioinspired electrodes demonstrate enhanced control over gas behavior.
Significant progress in understanding underlying mechanisms for improved performance.
Successful applications in hydrogen evolution reaction (HER) and carbon dioxide reduction reaction (CO2RR).

Conclusions:

Bioinspired gas manipulation is a powerful strategy for advancing electrochemical processes.
Further research into novel designs and mechanisms will unlock new applications.
Future work should focus on scalability and integration into practical electrochemical systems.