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Designing an Air-Stable Interphase on Lithium Metal Anode to Improve Cycling Performance.

Meng Yu1, Han Zhou1, Xiaohui Ning1

  • 1Center for Alloy Innovation and Design (CAID), State Key Laboratory for Mechanical Behavior of Materials, Xi'an Jiaotong University, Xi'an, Shaanxi 710049, P. R. China.

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|March 1, 2024
PubMed
Summary

Researchers developed an air-stable silver-fluoride interphase to protect lithium metal anodes (LMA) in rechargeable batteries. This innovation prevents dendrite growth, enhancing cycle life and safety for reliable energy storage.

Keywords:
air stabilityhybrid interphaselithium metal anode

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Energy Storage

Background:

  • Rechargeable lithium metal batteries (LMBs) face challenges with lithium dendrite growth, impacting cycle life and safety.
  • Uncontrolled dendrite formation leads to short circuits and potential hazards.

Purpose of the Study:

  • To develop an air-stable interphase for lithium metal anodes (LMA).
  • To improve the cycling stability and safety of LMBs by controlling lithium deposition.

Main Methods:

  • A facile solution-based approach was used to create an Ag-embedded fluoride-rich interphase.
  • Operando lithium plating experiments were conducted to observe lithium deposition.
  • Electrochemical performance was tested using a LiFePO4 cathode.

Main Results:

  • The Ag-F-rich interphase promoted uniform lithium nucleation and deposition, preventing dendrites.
  • The modified LMA demonstrated 300 stable cycles at 0.5 C with 91.4% capacity retention.
  • The interphase provided significant protection against air exposure, enabling over 120 cycles after 1 hour of air exposure.

Conclusions:

  • The functionalized interphase effectively protects the LMA from dendrite growth and air erosion.
  • This approach enhances the cycling performance and air stability of lithium metal batteries.
  • The developed interphase offers a promising strategy for advancing rechargeable lithium metal battery technology.