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High-Performance Flexible Ionically Conductive Superhydrophobic Papers via Deep Eutectic Polymer-Enhanced Interfacial

You Xu¹, Yunfeng Cao¹, Ren'ai Li¹

¹Jiangsu Co-Innovation Center for Efficient Processing and Utilization of Forest Resources, Jiangsu Provincial Key Lab Pulp & Paper Science and Technology, Nanjing Forestry University, Nanjing 210037, P. R. China.

Langmuir : the ACS Journal of Surfaces and Colloids

|March 14, 2024

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Researchers developed a superhydrophobic paper with flexible, conductive, and water-repellent properties. This innovation enhances paper-based electronics and smart sensing applications.

Area of Science:

Materials Science
Polymer Chemistry
Nanotechnology

Background:

Paper's limited conductivity and wettability restrict its use in advanced electronics.
Developing multifunctional paper for applications like green packaging and smart sensing is crucial.

Purpose of the Study:

To create a flexible, conductive, and superhydrophobic paper for advanced applications.
To investigate the role of deep eutectic polymers and fluorinated silica in imparting desired properties.

Main Methods:

A flexible transparent conductive substrate was fabricated using ethylcellulose and hydrophobic deep eutectic polymer via matrix swelling-polymerization.
Superhydrophobicity was achieved by modifying the substrate with fluorinated silica.
The material's electrical properties and response to deformation and water were characterized.

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Main Results:

The superhydrophobic paper exhibited an ultrahigh water contact angle (≈162.2°).
It demonstrated stable electrical sensing properties, responding to deformation/pressure with minimal impact from water.
The paper maintained stable electrical performance after 5000 bending-recovery cycles at 150°.

Conclusions:

The developed superhydrophobic paper offers a promising platform for flexible electronic devices.
The integration of deep eutectic polymers enhances energy dissipation, electrical sensing, and particle adhesion.
This work provides insights for designing advanced paper-based electronic devices.